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Keywords: The majority of operational liquefied natural gas (LNG) refueling stations in the world have no boil-off gas
Liquefied natural gas (BOG) management and rely on regular LNG delivery to condense the BOG. To reduce the pressure of LNG
Methane venting tanks onboard vehicles prior to filling, the BOG is vented to the atmosphere, is collapsed in the tank, or is
Boil-off gas management returned to the refueling station. In this study, different onboard LNG tank architectures are discussed, and the
Refueling station
design strategies for LNG conditioning and BOG management technologies employed in LNG refueling stations
Onboard LNG tank
Fuel supply system
are analyzed. The critical analysis of different designs of LNG refueling stations indicates that 44% of designs
have no BOG management, 28% of designs rely on liquid nitrogen condenser or a liquefier to condense the BOG,
and 28% of designs compress the BOG to produce compressed natural gas. Our research shows that in China
and the U.S., where stations with BOG management are rare, the number of LNG refueling stations has
increased by 32 and 3 times, respectively, between 2010 and 2015. This study highlights the fact that as heavy
fuel oil and diesel are replaced by LNG, it is critical to pay proper attention to the design of the LNG supply
chain and LNG refueling stations to minimize or eliminate BOG venting and reduce greenhouse gas emissions.
⁎
Corresponding author.
E-mail address: walter.merida@ubc.ca (W. Mérida).
http://dx.doi.org/10.1016/j.rser.2016.11.186
Received 13 April 2016; Received in revised form 26 September 2016; Accepted 12 November 2016
1364-0321/ © 2016 Elsevier Ltd. All rights reserved.
A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
Table 1
Methane emissions across different sectors.
Sector g methane/ m3 NG (vol%) GREET Model 2015 [41] g CO2 equivalent/ m3 NG Global Warming Potential [42,43]
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
study, we investigate different onboard LNG tank architectures, designs system (d) shown in Table 2). The pump is driven either electrically or
of LNG refueling stations, and mechanisms employed to manage and hydraulically. The pump pushes the LNG from the tank to the vaporizer
mitigate the BOG release rate. Also, we study current and future status and engine under any saturation conditions. It should be noted that
of LNG refueling stations in different countries. cryogenic pumps are generally expensive and the durability of compo-
nents can be problematic [45].
2. LNG refueling station and onboard fuel tank To prevent the pressure in onboard LNG tanks from exceeding the
fundamentals MAWP and BOG being released to the atmosphere, an economizer can
be added to the vehicle fuel supply system [45], as shown in Fig. 3. The
LNG tanks on vehicles or vessels are required to supply NG to the dashed box in Fig. 3 can be any of fuel supply systems (a)-(d) depicted
engine at the appropriate temperature, pressure, and flow rate. A in Table 2. The economizer permits a portion of BOG to be transferred
variety of strategies can be employed. In the simplest embodiments, the to the engine thereby removing energy from the tank and reducing its
fuel supply system relies on the pressure in the tank to provide pressure. This helps the pressure of the onboard LNG tank to remain
sufficient pressure to overcome the losses in the heat exchangers and below its MAWP and reset the LNG holding time of the fuel tank.
piping, and supply enough fuel to the engine. To improve fuel flow However, drawing the BOG, which is mainly composed of methane, for
performance, especially in the case of high-performance spark ignition sustained periods exclusively leaves the heavy hydrocarbons in the
engines, these simple onboard tanks are filled with so-called warm or LNG tank [38,45]. This enriched fuel with low methane content may
saturated fuel [45]. Saturated LNG has been heated prior to filling, to present problems for the engine when the economizer is disabled and
increase the saturation pressure, and therefore, supply the required the system switches back to conventional LNG fuel supply mode.
fuel flow rate. Other, more sophisticated tank systems are capable of Table 3 summarizes further advantages and limitations of fueling a
accepting so-called cold or unsaturated fuel which has not been pre- vehicle with saturated and unsaturated LNG.
conditioned. LNG dispensing systems at stations are therefore required To manage the BOG at high pressure in onboard LNG tanks, the
to provide unsaturated fuel, saturated fuel, and in some cases, super BOG should be 1) condensed by the unsaturated LNG during fueling, 2)
saturated (super warm) fuel, depending on the fuel supply system of vented to the atmosphere prior to fueling (an undesirable action), or 3)
the destination vehicle. transferred by a vapor return line to a station. In some tank designs,
Unsaturated LNG is dispensed at a less than −143 °C and 0.34 MPa this vapor return line is routed through the fill receptacle, e.g., Refs
(35 psig), and saturated LNG is dispensed at −125 to −131 °C, and 0.69 [48–51]., and in other designs, it is provided with its own connection,
to 0.93 MPa (85 to 120 psig) [39]. Unsaturated LNG has a higher e.g., Refs [52–56]. Therefore, the designs of LNG refueling stations and
density than saturated LNG, and as a result, more LNG can be stored dispenser equipment must accommodate these different vapor return
onboard with longer LNG holding time. However, the unsaturated fuel architectures. When an onboard LNG tank is required to be filled from
in an onboard LNG tank has a low pressure, and auxiliary equipment in a station, the operating sequence can be:
the vehicle fuel supply system are required to increase the fuel pressure
before it enters the engine. 1. No vapor back to station: Use the station pressure to overcome the
It was shown that fueling a vehicle with unsaturated LNG compared tank pressure and condense the BOG (only possible if the tank
to saturated LNG increases the driving range up to 12% and the LNG pressure has sufficient margin below the relief valve pressure and the
holding time from 5 to 10 days [46], as shown in Fig. 2. According to station pump has sufficient discharge pressure available).
SAE Standard J2343, the holding time of onboard LNG tanks in North 2. Vapor back to station: Use a vapor return line routed through the fill
America is 5 days [47]. Holding time refers to the time an onboard receptacle or a separate vapor return line to reduce the tank pressure
LNG tank holds the LNG without venting [30]. and then commence filling.
Table 2 shows different vehicle fuel supply systems with capability 3. Vapor back to station and continue to vapor back during fill
of running on saturated and unsaturated LNG. As shown in Table 2, operation (only possible with a separate vent return line): Transfer
system (a) is the simplest vehicle fuel supply system that operates only the LNG from the refueling station to an onboard LNG tank and the
by using saturated LNG. During fueling, LNG is sprayed from the top of BOG in the tank returns to the station by the vapor return line. In
the onboard LNG tank to condense the existing BOG at high tempera- this method, the LNG pressure at the station does not need to be too
ture. During operation, the LNG is transferred by the pressure gradient high.
from the higher pressure tank to the vaporizer and engine [38,45].
However, this fuel supply system may not be able to sustain full fuel The BOG returned from onboard tanks to refueling stations mixes
flow at continuous high fuel demand. with the BOG produced by the LNG station, and to prevent venting, it
Vehicle fuel supply system (b) shown in Table 2 is equipped with a should be condensed by an onsite LNG liquefier, liquid nitrogen (LN2)
pressure-building circuit. The pressure-building circuit evaporates a condenser, or be purged to a pipeline nearby the station with a
portion of LNG to increase the BOG pressure in the vapor space and
create a pressure gradient between the tank and the engine [45]. Using 1250 11
this fuel supply system, LNG does not require to be conditioned at the Driving range 10
Holding time 9
LNG holding time (day)
refueling station. However, this fuel supply system has two technical 1200
Driving range (km)
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
Table 2
Different vehicle fuel supply systems and their capability of running on saturated and unsaturated LNG.
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
Table 3 Table 4
Advantages and limitations of fueling onboard LNG tanks with saturated and Comparison of LNG bulk and on-the-fly conditioning [45].
unsaturated LNG.
LNG bulk conditioning
Saturated LNG fueled in onboard tanks with a simple architecture [45]
Advantages Limitations
Advantages Limitations • Straightforward, simple, and • Mass of fuel stored in the station is reduced.
• Fueling system is simple, reliable, • Fuel conditioning at station increases robust. • LNG holding time is reduced and risk of
durable, and less expensive. station cost and complexity. • Fully proven and is in venting is increased.
• Lower fuel density and shorter driving
range.
common use. • Cannot
vehicles.
deliver unsaturated LNG to
engine.
Unsaturated LNG fueled in onboard tanks with a pump [38] and on-the-fly conditioning. Fig. 4a shows a simplified schematic of a
Advantages Limitations
• Does not need fuel conditioning
at station.
•
Pump is needed.
LNG refueling station with bulk conditioning. The refueling station is
comprised of a storage tank, sump tank, pump, heater, dispenser, and
• Denser low-pressure fuel and
longer driving range.
vapor return line. After filling the storage tank, the pump sends the
LNG to the heater to rise its temperature and pressure. This process
• Provides longer LNG holding
time.
continues until the LNG pressure stored in the storage tank reaches a
set point.
In contrast, a LNG refueling station with on-the-fly conditioning
increases the pressure and temperature of LNG simultaneously with
and can also deliver LNG to vehicles if equipped with a LNG dispenser. the fueling process, as shown in Fig. 4b. This method helps the storage
Combined LNG/LCNG refueling stations are capable to deliver CNG to tank to store more LNG with higher density for a longer time. However,
light- and medium-duty vehicles, and LNG to heavy-duty vehicles. the heater needs to be precisely designed to heat the LNG on-the-fly
Also, they have lower capital and operating costs than similarly sized within a short time without adding too much heat. Linde North
CNG refueling stations [59]. However, high-pressure reciprocating America Inc. designed and installed the first generation of LNG
LNG pumps used to generate the CNG require extended cooldown refueling stations with on-the-fly conditioning in the U.S. in 2014
time which generates significant quantities of BOG. This BOG must [61]. Further information about advantages and limitations of LNG
then be processed using a compressor and added to the CNG reservoir. bulk and on-the-fly conditioning are summarized in Table 4.
The compressor can also compress the BOG generated in the LNG Currently, several vendors are involved in the design and installa-
storage tank and the BOG returned from vehicles to produce CNG. tion of LNG and LCNG refueling stations. NorthStar, Inc. (Clean
To fuel vehicles with different fuel supply systems, LNG refueling Energy) [62], Chart Industries [63], CryoStar [64], ENN Canada
stations filled with unsaturated LNG should be able to deliver saturated [65], and Linde Group [66] are the main suppliers of LNG and
LNG by conditioning the unsaturated LNG. LNG conditioning is a LCNG stations with different technologies. Fig. 5 shows schematics of
process in which temperature and pressure of LNG increase to meet set LNG and LCNG refueling stations manufactured by Chart Industries. It
values. Two methods of LNG conditioning at refueling stations are bulk can be seen in Fig. 5a that the LNG refueling station has a heater for
Fig. 4. LNG conditioning at a refueling station: (a) bulk conditioning method [45] and (b) on-the-fly conditioning method [60].
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
Fig. 6. Schematic of a LNG refueling station with on-the-fly conditioning and LN2 The vast majority of LNG refueling stations are distributed along
condenser manufactured by Linde North America Inc [61].
the roads where heavy-duty vehicles travel. There are a limited number
of LNG refueling stations for inland waterway vessels and off-road
LNG bulk conditioning with no BOG management. This is the simplest vehicles. Table 6 shows the existing and proposed LNG refueling
and probably the most economical LNG refueling station design. As stations for on-road vehicles in different countries. China has the
shown in Fig. 5b, an LCNG refueling station is equipped with a high largest number with 3,200 LNG refueling stations [74] followed by the
pressure pump to increase the LNG pressure, a vaporizer to convert U.S. with 122 LNG stations [75]. The total number of LNG stations in
LNG to CNG, and a CNG buffer storage tank to store the CNG for Europe is currently 46 and 6 more stations are either proposed or are
fueling vehicles. currently under construction in Portugal, France, and Italy.
A schematic of LNG refueling station with on-the-fly conditioning The rate of LNG deployment varies around the world. Fig. 8
and an LN2 condenser manufactured by Linde North America Inc. is indicates that in China, the number of LNG refueling stations has
shown in Fig. 6. This station can manage the BOG if LN2 is regularly increased from 100 in 2010 to 3200 in 2015 (a 32 fold increase) [74]. It
supplied to the refueling station. is expected that the number of LNG refueling stations in China will
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
Table 5
Different designs of LNG refueling stations reported in the literature.
Cieslukowski [48] No loss single-line LNG • Storage tank • Conditioning in the • It can deliver LNG at • Complex design for the sump tank
refueling station • Sump tank with a sump tank different pressures and and fuel delivery system
flexible roof • Single line for vapor temperatures • No pump to overcome the pressure of
• Liquefier
tank)
(LN2 return and LNG
fueling
• It conditions LNG on
demand
the remainder of BOG in the onboard
LNG tank
• Saturation coils • Delivering saturated • It can liquefy the BOG • management
High dependency on LN for the BOG
• Single fueling line
2
LNG
Gustafson [67] No loss LNG refueling • Storage tank • LNG bulk • It precools the pump and • The eductor cannot effectively remove
station • Centrifugal pump conditioning pipes by recirculating LNG the BOG at low LNG flow rates
• Eductor • Vapor collapse • It removes a portion of the • The pump and pipes are in direct
• Saturation coils method BOG generated in the LNG contact with the environment leading
• Flowmeter • Delivering saturated storage tank by the eductor to high heat transfer to LNG over time
LNG • Single fueling line • No reliable BOG management
Goode [52] LNG refueling station and • Storage tank • LNG bulk • It precools the pumps and • ItThehaspump
a sophisticated control system
its control system • Centrifugal pump conditioning pipes by circulating LNG • the environmentand pipes are exposed to
• Saturation coils • Vapor return method causing extra heat
• Flowmeter • Delivering saturated transfer to LNG
LNG • No BOG management
Kalet and LNG refueling station and • Storage tank • conditioning
LNG on-the-fly • It delivers unsaturated LNG • Itwhich
requires an overflow tank on vehicle
Gustafson [68] configuration of vehicle • Pump to collapse the BOG and then adds to the cost, complexity of
onboard fuel tanks • Vaporizer • Vapor collapse vaporizes LNG to increase fueling system, and weight of vehicle
• Pressure transducer method the pressure of onboard • ItLNGrequires high power to vaporize
• Microprocessor • Delivering saturated LNG tanks within a short time to increase
• tank
Vehicle overflow and unsaturated • Single line fueling the onboard LNG tank pressure
LNG • No BOG management
Powars [69] LNG refueling station • Storage tank • No conditioning • BOG management • The LNG refueling station only
driven by LN2 • LN tank • Vapor collapse • Single line fueling operates with LN
• LN vaporizer • for
2 2
method LN is directly in contact with LNG
• Delivering
2 2
condensation of BOG and
unsaturated LNG generating pressure
• No LNG recirculation in the LNG
storage tank which causes LNG
stratification
Barclay [53] LNG and CNG refueling • LNG liquefier • conditioning
LNG on-the-fly • It converts NG to LNG onsite • It requires a NG supply pipeline with
station with onsite LNG • Vaporizer • BOG management enough pressure
liquefier • Storage tank • Vapor return method • It has high construction costs due to
• Expander • Delivering saturated onsite liquefier, two vaporizers, and
• Pump and unsaturated an expander
• CNG buffer tanks LNG • Itandliquefies the NG to produce LNG
then convert LNG to CNG. This
process increases the energy
consumption of the station
Gustafson and No loss LNG and CNG • Storage tank • LNG conditioned in • The compressor can remove • The CNG compressor is expensive. As
Kalet [57] refueling station • Two LNG
conditioning tanks
two conditioning
tanks
the BOG from storage tank
and reset the LNG holding
an alternative, a high pressure pump
can be used.
• Vaporizer • Vapor collapse time • It requires a precise control system to
• Saturation coils method • CNG is used to increase the adjust pressures in different parts of
• Compressor • Delivering saturated pressure and temperature of the station because there is no pump
• Flowmeter and unsaturated LNG in the conditioning in the design
• CNG buffer tanks LNG tanks • It has high construction costs due to
compressor, vaporizer, saturation
coils, and two conditioning tanks
Dehne [54] Zero-vent LNG refueling • Three storage tanks • LNG bulk • It can deliver saturated and • It requires 3 storage tanks of the same
station • Pump conditioning unsaturated LNG size which add capital costs
• Saturation coils • Vapor return method • It stores significant amount of
• Delivering saturated
and unsaturated
conditioned LNG for a long time that
contributes to BOG generation
LNG • No BOG management
Preston et al. [70] Self-contained LNG • Storage tank • LNG bulk • It is a mobile system • No BOG management
refueling station • Sump tank conditioning • No precooling is required.
• Saturation coils • Vapor collapse The pump and flowmeter
• Pump method are submerged inside the
• Flowmeter • Delivering saturated LNG sump tank
LNG • Single fueling line
Forgash et al. [49] Four different designs for • Storage tank • LNG bulk • It uses a compressor to • Using compressor adds to the station
Kooy et al. LNG refueling station • Pump conditioning remove the BOG from LNG cost and maintenance
[50] • Saturation coils • Single line for vapor storage tank and purge it to • The BOG removed from the LNG
• Compressor return and LNG LNG fueling line onboard tank flows only by pressure
• Flowmeter fueling gradient which may not be enough to
• Sump
(recommended)
tank • Delivering saturated
and unsaturated
remove the BOG properly
LNG
(continued on next page)
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
Table 5 (continued)
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A. Sharafian et al. Renewable and Sustainable Energy Reviews 69 (2017) 503–513
100 100
Fuel supplied by refueling station BOG status in onboard LNG tank in refueling process
90 90
80 80
% of refueling stations
% of refueling stations 72%
70 70
60 60 55%
50 50
40 40
28% 28%
30 30
20 20 17%
10 10
0 0
LNG LNG + CNG Vapor collapse Simultaneous vent to Vent through the fill
station while filling line in advance of filling
(a) (c)
100 100
LNG conditioning status at refueling station BOG management status at refueling station
90 90
BOG management by liquefier (LN2)
80 80
% of refueling stations
% of refueling stations
No
BOGBOG management
management by CNG production
70 70
60 60 56%
50 50 44%
40 33% 33% 40 28%
30 30
20 17% 17% 20
10 10 28%
0 0
Bulk conditioning Conditioning in LNG on-the-fly No conditioning BOG management No BOG management
sump tank or conditioning
secondary tank
(b) (d)
Fig. 7. Comparison of different refueling station designs in terms of (a) delivering LNG or LNG and CNG, (b) conditioning LNG at refueling station, (c) managing the BOG in onboard
LNG tank, and (d) managing the BOG at refueling station.
Table 6 reach 5000 by 2020. In the U.S., the number of LNG refueling station
Number of existing and proposed LNG refueling stations by country. gradually increased between 2010 and 2015 [79]., as shown in Fig. 8.
The number of LNG refueling stations in the U.S. increased from 40 in
Country Existing LNG LNG Stations proposed or Ref.
Stations under construction
2010 to 122 in 2015 (a 3 fold increase) and 54 more LNG refueling
stations are either proposed or are currently under construction.
China 3200 1800 [74] Based on this analysis and the number of LNG refueling stations
USA 122 54 [75] discussed, it can be concluded that LNG usage in the transportation
Canada 12 – [6]
Spain 12 – [76]
sector is increasing and will continue in the next decade. Equipment
Netherland 12 – [76] design along the LNG distribution chain will play a major role. New
Australia 10 – [77] scenarios in BOG management of LNG refueling stations and vehicles’
United Kingdom 9 – [76] onboard LNG tanks should be implemented to get short- and long-term
Sweden 7 – [76]
benefits of switching from conventional petroleum fuels to LNG.
Belgium 2 – [76]
Portugal 2 3 [76]
France 1 2 [76] 5. Conclusions
Italy 1 1 [76]
Japan 1 – [78]
LNG can replace diesel in heavy-duty vehicles, ships, and trains.
However, the unintended release of methane (the main constituent of
LNG) contributes more than CO2 to climate change in a 20-year
6000 horizon. Methane emission analysis across the supply chain indicated
No. of LNG refueling stations in U.S.
No. of LNG refueling stations in China
5000
China 140 that transportation, storage, and distribution sectors are the largest
122
5000 U.S. contributors to these fugitive emissions. LNG refueling stations and
120
vehicles’ onboard LNG tanks are the main parts of the distribution
103
4000 100 sector. Our analysis showed that BOG management in LNG refueling
3200
80 different fuel supply systems, and minimizing heat transfer to the LNG
2500
3000
61
60 between the storage tank and dispenser were parameters that needed
1844
1000
20
200
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