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Formation of a laccolith by magma pulses: Evidence from modal and


chemical composition of the 500 m long borehole section through the Permo-
Carboniferous Landsberg laccolith (Halle...

Article  in  Geochemical journal GJ · September 2015


DOI: 10.2343/geochemj.2.0382

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Geochemical Journal, Vol. 49, pp. 523 to 537, 2015 doi:10.2343/geochemj.2.0382

Formation of a laccolith by magma pulses: Evidence from modal and chemical


composition of the 500 m long borehole section through
the Permo-Carboniferous Landsberg laccolith (Halle Volcanic Complex)

·
ELZBIETA SL ODCZYK ,1* ANNA PIETRANIK,1 CHRISTOPH BREITKREUZ,2 ARTUR P˛EDZIWIATR,1 MARCIN BOKL A ,1
KATARZYNA SCHAB 1 and MARTA GRODZICKA1

1
Institute of Geological Sciences, University of Wroc l aw, ul. Cybulskiego 30, 50-205, Wroc l aw, Poland
2
Institute for Geology and Paleontology, Bernhard-Von-Cotta-Str. 2, TU Bergakademie, Freiberg, Germany

(Received March 9, 2015; Accepted June 19, 2015)

The 500 m long section through the upper part of the Permo-Carboniferous Landsberg laccolith (Halle Volcanic Com-
plex) was sampled every 25 meters. The modal proportions between plagioclase and K-feldspar phenocrysts vary in the
section and the laccolith may be divided into four parts with different proportions of Pl/Kfs, which, in subvolcanic rocks,
should reflect different proportions of these minerals in the magma plumbing system. Chemical composition of whole
rock samples is uniform, but the correlations of Si and other elements with depth within all of the four sections suggest
that the sections based on modal composition are also reflected in chemical composition of the rock. Also, the uppermost
100 meters of the laccolith has slightly higher contents of Fe, Ti, Zr and Nb compared to those in the rest of the laccolith
and this is consistent with it being a separate magma pulse derived from a distinct source. Detailed analyses of chemical
variations within each section are consistent with the model that the upper 500 meters of the Landsberg laccolith was
formed by three successive pulses with slightly different chemical compositions. The best documented is the uppermost
pulse, which was over-accreted on the first pulse. Another pulse was probably emplaced in the middle of the first pulse.
The thickness of the pulses was 100–300 m, which is consistent with previous 2D and 3D emplacement models of the
Halle laccoliths. However, the contacts between the pulses based on modal and chemical compositional variations are not
always concurrent with the presence of shearing zones, the discrepancy that is not yet well understood. In general, be-
cause silica-rich laccoliths are relatively small bodies that cool quickly due to high level of emplacement, they may
preserve better evidence for separate magma pulses compared to plutonic batholiths.

Keywords: laccolith formation, magma pulses, rhyolite, Halle Volcanic Complex

INTRODUCTION variations in layering (Pons et al., 2006), or could be rec-


ognized only later by differences in chemical composi-
Recent field, geochemical and mineralogical studies
tion between the pulses (e.g., Wiebe et al., 2002; Matzel
show that magma chambers develop and grow by amal-
et al., 2006; Michel et al., 2008). However, chemical vari-
gamation of several intrusions (Coleman et al., 2004;
ations within the magma body could also be an evidence
Horsman et al., 2009). The process was documented for
for fractional crystallization and/or magmatic segregation.
both deep-seated granitic plutons (e.g., Glazner et al.,
Additional information that may help to indicate that in-
2004) and also for subvolcanic laccoliths (e.g., Mock et
ternal heterogeneity in the magma body was due to sepa-
al., 2003). The style of magma emplacement depends on
rate magma pulses can be provided by application of quan-
the size and form of a magmatic body and many other
titative textural analysis including modal abundance of
important variables such as depth, wall-rock structure,
minerals (Mock et al., 2003).
magma viscosity. Sills grow mainly by lateral propaga-
In the current paper we use combined chemical and
tion, whereas laccoliths seem to grow by vertical thick-
mineralogical analyses of selected samples from the 500
ening before extending laterally again to form plutons and
m long completely cored well, which constitutes the up-
batholiths (Menand, 2008). The separate pulses forming
per part of the coarse-grained rhyolitic Landsberg
laccoliths or plutons could be observed in the field due to
laccolith (Halle Volcanic Complex, Germany). The bot-
tom of the laccolith was not drilled, but the core analysed
in this paper probably represents more than half of the
*Corresponding author (e-mail: elzbieta.slodczyk@ing.uni.wroc.pl)
vertical section through the laccolith. Our goal is to in-
Copyright © 2015 by The Geochemical Society of Japan. terpret the modal and chemical variations of the Landsberg

523
are in accordance with the 3D emplacement model of the
Landsberg laccolith suggested by Schmiedel et al. (2015).

GEOLOGICAL S ETTING
Voluminous magmas of felsic to mafic composition
were formed across Central Europe at the Carboniferous/
Permian transition (Romer et al., 2001; Breitkreuz et al.,
2007; Oberc-Dziedzic et al., 2010; Turniak et al., 2014).
Chemical characteristics suggest that this magmatism was
caused either by mantle upwelling in a post-collisional
setting (e.g., Zeh et al., 2000; Turniak et al., 2014), or by
ongoing plate subduction (Schmidberger and Hegner,
1999). However, the subduction-type chemical charac-
teristic are probably inherited from the melting of crust,
which was affected previously by subduction-related flu-
ids (Romer et al., 2001). Halle Volcanic Complex (HVC)
was formed during the Permo-Carboniferous magmatic
activity and consists of several laccoliths located in the
Mid-German Crystalline Rise (MGCR), in the northeast-
ern Saale Basin in eastern central Germany (Romer et
al., 2001; Mock et al., 2005; Breitkreuz et al., 2009). The
magmatic activity of the HVC is characterized by silica-
rich, shallow emplaced units (~300 km 3, Mock et al.,
2005; Schmiedel et al., 2015) forming three fine-grained
porphyritic (Wettin, Petersberg and Brachstedt) and two
coarse-grained porphyritic laccoliths (Löbejün and
Landsberg; Fig. 1, Breitkreuz and Mock, 2004; Mock et
al., 2005; Schmiedel et al., 2015). The coarse and fine
grained laccoliths have also different aspect ratios (height
to length), approximately 0.07 for coarse grained and 0.04
for fine grained units (Schmiedel et al., 2015).
The intrusive character of the laccoliths is confirmed
by their large thickness, tilting of bedding in sedimen-
tary rocks occurring between the laccolith units and the
presence of internal flow structures within the units (Mock
et al., 2003). The three types of margin geometries dis-
tinguished within HVC laccoliths include (1) vertical
margin of an intrusive-extrusive complex visible in
Löbejün laccolithic unit; (2) stacked lobes/fingers for
Fig. 1. a) Distribution of coarse and fine grained rhyolitic Petersberg and Brachstedt units; (3) sediment rafts en-
laccolith units within Halle Volcanic Complex. Inset shows the
gulfed by rhyolitic sheets within Landsberg unit (for de-
location of the study area within Germany; b) corresponding
a–b cross section; c) location of the investigated drill core
tails and source literature see: Schmiedel et al., 2015).
within Landsberg laccolith; figures modified after: Breitkreuz Overall geometry of the HVC is well documented by about
and Mock, 2004; Mock et al., 2005; Schmiedel et al., 2015. 6000 wells, some of which reaching down to 700 m depth.
3D modeling of the Landsberg unit estimated its mini-
mum volume at ~63 km3 (Schmiedel et al., 2015).
The coarse grained Löbejün and Landsberg laccoliths
laccolith in the context of recent models of pulsed magma are composed of porphyritic rhyolite with large feldspar
chambers formation. We particularly seek to provide com- phenocrysts up to ~30 mm long (Mock et al., 2003), and
plimentary information on the magma chambers forma- with zircon SHRIMP ages of 297 ± 3 Ma and 301 ± 3 Ma
tion, which may come from relatively quickly chilled respectively (Breitkreuz and Kennedy, 1999; Breitkreuz
laccoliths and may be lost in longer-lived plutons. In de- et al., 2009). The Wettin, Petersberg and Brachstedt
tail, we aim to check if geochemical and petrological data laccoliths are composed of fine-grained porphyritic

524 E. S l odczyk et al.


rhyolite and have zircon SHRIMP ages of 297 ± 3 Ma, topic composition of K-feldspar indicates involvement of
292 ± 3 Ma and 292 ± 3 Ma, respectively (Breitkreuz and isotopically distinct sources (crustal and mantle) (Romer
Kennedy, 1999; Breitkreuz et al., 2009). These rhyolite et al., 2001) and similar conclusion is supported by eHf
units contain small (~10 mm) feldspar phenocrysts, which and d 18O in zircons, which show relatively uniform, but
define textural variations (Mock et al., 2003). scattered values (eHf = –4.1 to –8.4 and d18O = 6.4 to
8.3, Sl odczyk et al., in revision). Hf and O isotopes in
Geochemistry of the HVC: previous research zircon are similar between different laccolith units, but
All major rock types forming the HVC were investi- they are consistent with derivation of the magmas form-
gated by Romer et al. (2001) who presented major and ing the laccoliths from several different sources. In de-
trace element data as well as Sr and Nd isotope composi- tail, the variability of Hf and O isotopes in zircon sug-
tions for felsic, intermediate and mafic rocks. K-feldspar gests remelting of heterogeneous crust with minor to neg-
phenocrysts from rhyolite units were also analysed for
ligible contribution from the mantle (S l odczyk et al., in
Pb isotopes (Romer et al., 2001), and Hf and O isotopes
revision). It is also clear, based on zircon analyses, that
in zircon were analysed in both fine grained and coarse
the rhyolites evolved in at least two stages, with the last
grained rhyolites (S l odczyk et al., in revision). stage being remelting of crystal mush or a granite batholith
Mafic and intermediate rocks of the HVC were formed shortly prior to the rhyolites formation (a similar
grouped by Siegert (1967a, b) into four groups of model was also suggested by Bryan et al. (2008), Pietranik
Porphyrites (I–IV) with decreasing age of emplacement et al. (2013)).
and Romer et al. (2001) analysed samples from these
groups. The rock types analysed in each group included Quantitative textural analyses of finely grained
trachybasalts of Porphyrite I group, trachyandesites and Petersberg laccolith: previous research
trachydacites of Porphyrite II and IV groups and basaltic The knowledge about 3D geometry and stratigraphy
trachyandesites of Porphyrite III group. Generally, the of the HVC comes from natural outcrops and deep wells.
samples are strongly altered and, therefore, the concen- Analyses of internal structures and textures from the top
trations of the mobile elements (such as MgO, CaO, Na2O, to the bottom of laccoliths show changes in the size and
K2O, Li, Rb, Sr, Zn, Cs, Ba, Pb, U) are affected and could packing arrangement of the phenocrysts with depth (Mock
be used only in a limited way (Romer et al., 2001). Based et al., 2003).
on Sr and Nd isotope composition, the Porphyrites were Petersberg laccolith forms one the largest laccoliths
divided into two groups: (1) less evolved Porphyrites I in the HVC (~60 km3) and has been sampled at six differ-
and II (eNd (T=300Ma)= –0.8 to –1.7; 87Sr/ 86Sr (T=300Ma) = ent depths of 49.9 m, 167.1 m, 184.3 m, 223.5 m, 250.8
0.7053–0.7060); and (2) more evolved Porphyrites III and m, 286 m (Mock et al., 2003). Modal abundances of
IV ( e Nd (T=300Ma) = –5.9 to –7.4; 87 Sr/ 86Sr (T=300Ma) = orthoclase (Or), plagioclase (Pl) and quartz (Qtz)
0.7065–0.7094). phenocrysts were similar in each sample. The detailed
Felsic rocks in the HVC comprise rhyolites that are analysis of crystal population showed: (1) continuous
low-Si (SiO2 = 71.5–72.5 wt%), calc-alkaline (K2O/Na2O growth of crystals in the magma during its ascent and
= 1.7–1.9) and weakly peraluminous (A/CNK = 1.04– emplacement (determined by crystal size distribution); (2)
1.08). Characteristic feature for all of the rhyolites is their flow alignment of feldspar crystal as a result of flow shear-
uniform contents of Zr, Hf, REE, Nb, Ta, Th, TiO2, and ing; (3) redistribution of crystals as a result of the flow;
P2O5 (Romer et al., 2001). Differences in some other trace (4) emplacement of the laccolith involving successive
elements may be explained by postmagmatic alteration pulses of magma intruding each other (determined by
and surface weathering (Romer et al., 2001). For exam- spatial distribution of phenocrysts); (5) distinct (two?)
ple Li, Rb, Cs and Zn decrease during chloritization of magma pulses that contributed to the growth of the
biotite while Ca, Sr, and Pb depletion is linked to laccolith. In this study we combined both whole rock
albitization (and weathering) of feldspars (Romer et al., geochemistry and modal abundances of phenocrysts to
2001). Nd isotope composition of rhyolites is also uni- see if similar laccolith formation processes are recorded
form and similar to Porphyrites III and IV (eNd(T=300Ma) for coarse grained rhyolite variety forming the Landsberg
= –6.7 to –7.0). In contrast, Sr isotope composition is more laccolith.
variable and higher than that of the Porphyrites (87Sr/
86
Sr(T=300Ma) = 0.7100–0.7128), but Sr isotopes could also
have been altered by post-magmatic processes. Isotope METHODS
composition (Sr, Nd, Pb) of K-feldspar phenocrysts is Rock samples were taken from the fully preserved 500
similar to that of the whole rock, but with more variable m drill core representing the upper part of the Landsberg
Sr isotope composition (87Sr/86Sr(T=300Ma) = from 0.7107– laccolith (the unit has never been perforated by wells,
0.7108 to 0.7044–0.7065, Romer et al., 2001). The iso- even the deepest one having 710 m), stored in the Geo-

Landsberg laccolith formed by magma pulses 525


Fig. 2. (a) Representative fragment of the drill core, (rhyolite from 29 m depth); (b–d) representative microscope images of the
analysed rhyolite (crossed polarized light).

526 E. S l odczyk et al.


Table 1. Modal composition of samples from the Landsberg laccolith

Sample depth [m] Minerals Background Pl/Kfs Section


Qtz Pl Kfs Opx*
29 9.3 13.2 9.6 2.1 65.8 1.4 1
56 7.7 13.4 8.0 2.7 68.2 1.7 1
76 6.0 14.2 11.3 2.4 66.1 1.3 1
102 9.9 14.1 9.2 2.3 64.5 1.5 1
102 8.7 12.7 14.2 1.7 62.7 0.9 2
128 6.8 12.2 14.8 3.3 62.9 0.9 2
155 10.6 8.6 12.6 2.9 65.3 0.7 2
175 7.2 12.4 16.4 3.5 60.5 0.8 2
197 8.3 11.4 14.2 3.7 62.4 0.8 2
201 9.5 13.1 8.2 3.2 66.0 1.6 3
225 10.7 9.6 13.7 2.6 63.4 0.7 3
245 12.3 10.8 9.3 3.7 63.9 1.2 3
258 8.8 8.6 15.5 2.8 64.3 0.5 3
281 8.8 13.8 12.4 3.9 61.1 1.1 3
281 7.7 7.4 17.7 2.2 65.0 0.4 3
304 8.9 14.3 10.4 1.9 64.5 1.4 3
357 6.9 10.2 18.2 1.8 62.9 0.6 3
378 8.6 8.8 9.7 3.5 69.4 0.9 4
400 9.2 11.2 13.5 4.5 61.6 0.8 4
452 8.2 10.4 12.4 2.1 66.9 0.8 4
481 8.9 13.5 11.3 4.2 62.1 1.2 4

*Opx is often replaced by opaque minerals.

logical Survey of Sachsen-Anhalt in Halle. It can be esti- Additionally, cathodoluminescence (CL) images of
mated that the 500 m represents more than half of the quartz were done for thin sections from 16 m and 490 m.
laccolith vertical section as based on the aspect ratios of The thin sections were carbon-coated, and analysed us-
other laccolith units in the area. We sampled the rhyolite ing a “hot cathode” CL microscope HC1-LM (cf., Neuser
drill core approximately at 25 m intervals taking samples et al., 1995). The system was operated at 14 kV acceler-
of 4 cm-diameter core from 15 up to 30 cm in length. The ating voltage and a current of 0.2 mA (current density of
most fresh looking samples were chosen for this study, about 10 mA/mm 2). Luminescence images were captured
however, most samples contained phenocrysts affected “on-line” during CL operations using a peltier cooled,
by secondary processes. The samples were cut vertically digital video-camera (OLYMPUS DP72).
to show flat rectangular surface, which was scanned to Major and trace elements were analysed in all sam-
obtain high quality images. Additionally thin sections ples in the ACME laboratories. Major elements were ana-
were prepared from 3 depths: 16 m, 250 m and 490 m lysed by ICP-ES, whereas trace elements by ICP-MS.
representing the top, the middle and the bottom of the Accuracy of the data was checked by replicate analysis
preserved drill core. The samples were described and the of STD SO-18 reference material (n = 2) (Supplementary
images were analysed in JMicroVision freeware Table S2) and it is below 1% for SiO2, Al2O3, Fe2O3, MgO,
(www.jmicrovision.com/index.htm). The program was CaO, MnO and below 7% for Na2O, K2O, TiO 2, P2O5,
used for measuring and quantifying components of high- Cr2O3. Reproducibility was checked for 3 samples, which
definition images, including scans and thin sections. To were analysed in replicates. It was less than 5% for all
maintain larger analysed surface and, thus more repre- the major elements with the exception of CaO. Repro-
sentative quantitative data from different drill core depths, ducibility for trace elements was also less than 5% apart
we only used samples with surface area between 10 and from Sm, Eu, Dy, Ho, Tm.
50 cm2. To check on the reproducibility of the results the
analyses of some cores were done in replicates (Supple- RESULTS
mentary Table S1). Differences were usually less than 5%.
The accuracy was limited by the macroscopic recogni- Petrography and modal composition
tion of minerals by human eye, therefore the results were All the analysed samples of the coarsely porphyritic
double checked by analyzing thin section from the same Landsberg rhyolite have similar mineral composition and
depths. contain phenocrysts of K-feldspar (Kfs), plagioclase (Pl),

Landsberg laccolith formed by magma pulses 527


Fig. 3. (a) Variations in Pl/Kfs proportion with depth and a first-hand interpretation linking the variations in the Pl/Kfs ratio
with separate pulses (see also text); (b–g) variations in chemistry within 500 m drill core of the Landsberg laccolith.

quartz (Qtz) and a mafic phase orthopyroxene (Opx) and/ vided the drill core in 4 sections from the top to the bot-
or biotite (Bt) (Fig. 2a). The largest phenocrysts are K- tom: (1) Section 1: Pl dominates with relatively high Pl/
feldspar with the longest dimensions usually from 0.5 cm Kfs ratios from 1.3 to 1.7. (Table 1); (2) Section 2: Kfs
up to several cm (Fig. 2b). Plagioclase is usually smaller dominates with low Pl/Kfs ratio from 0.6 to 0.9; (3) Sec-
from 2 mm to 1 cm. Background is fine grained (~0.1 tion 3: variable proportion of Pl and Kfs with Pl/Kfs val-
mm) and composed of quartz, feldspars and opaque min- ues form 0.4 to 1.6; (4) Section 4: Kfs dominates with
erals (Figs. 2b–d). Feldspars and mafic minerals are usu- relatively low Pl/Kfs ratios, mainly below 1.
ally fully replaced by secondary minerals e.g., sericite in
feldspars (Fig. 2b) and opaque minerals in orthopyroxene Geochemical data
(Fig. 2d). Generally, despite the alteration, the major min- Major and trace element contents in rhyolites are simi-
erals could be distinguished in most of the analysed cores. lar between the samples and also typical for rhyolites from
Only the cores at depths 328 and 428–430 m were thor- the HVC as reported by Romer et al. (2001). All the sam-
oughly altered and the recognition of the minerals was ples from Landsberg laccolith have similar composition
not possible (Table S1). Despite general similarity in min- in CHUR normalized REE diagrams and primitive man-
eral composition and texture, the rhyolite shows differ- tle normalized spider diagrams. They show LREE en-
ences in the relative abundances of phenocrysts and riched chondrite-normalised REE patterns and negative
groundmass (Table 1; Table S2), with the most pro- Eu anomaly (Fig. 4a). Also all rhyolites (coarse and fine
nounced being relative proportions of K-feldspar and grained types) form the HVC, including these analysed
plagioclase (Fig. 3a). Based on these differences we di- in this study, overlap in the same compositional field in

528 E. S l odczyk et al.


Fig. 4. (a) Chondrite-normalised REE patterns of Landsberg rhyolite (dark, this study) and rhyolite from HVC (grey, Romer et
al., 2001). Chondrite data from McDonough and Sun, 1995; (b) trace element patterns for Landsberg rhyolite normalized against
primitive mantle (McDonough and Sun, 1995); (c, d) selected trace elements versus 1/TiO2.

the 1/TiO2 vs. Zr and Y (Figs. 4c and d respectively). ples from this section and those from other sections (one-
Consistently lower Ca, Sr and Pb contents of Landsberg way ANOVA test, P < 0.05, post-hoc Pairwise Multiple
rhyolites compared to unaltered fine grained rhyolites Comparison Procedure, Holm-Sidak method). Similar
analysed by Romer et al. (2001, Fig. 4b) indicate that high contents of Sr, Ti, Zr and Nb occur also in selected
plagioclase alteration could have affected the chemical samples from Section 3 (Fig. 3) and these samples have
composition of the whole rocks. Consequently, the po- also higher proportions of Pl/Kfs similar to those observed
tentially mobile elements can not be used for interpreta- in Section 1 (Fig. 6).
tion of chemical variability of the Landsberg rhyolites. Correlations with the depth for the whole laccolith
Generally, Landsberg samples have uniform compo- section are weak (R2 = 0.0 for P 2O 5 to 0.39 for Fe2O3).
sition, however, in detail, distinct variations in composi- However, some correlations in chemical composition can
tion between samples were observed. Twenty one sam- be related to the different sections distinguished in the
ples from the Landsberg laccolith are characterized by a laccolith based on the Pl/Kfs ratio (Fig. 3a). For exam-
range of SiO 2 contents from 71.5 to 73.8 wt% with only ple, Si content decreases with depth in Sections 1, 3 and
one outstanding sample (SiO2 = 67.7 wt%). Compositional 4 (R2 = 0.64, 0.88 and 0.85 respectively) and increases
variations within sections defined by different Pl/Kfs ra- with depth in Section 2 (R2 = 0.77, Fig. 3b). The low Si
tios are small, but samples from Section 1 (the upper- sample occurs at the border between Sections 2 and 3.
most 100 m) are characterized by the lowest CaO and For many elements, e.g., Si, Al, K and Na Sections 2 and
MgO (Table 2) and the highest, FeO, TiO2, K2O, Ba, Sr, 4 show opposite trends with depth (Fig. 5). Section 1
Zr, Nb, Rb (Figs. 3c–g, Table 2). There is a statistically shows strong negative correlations with depth for LREE
significant difference in Fe and Ti contents between sam- (e.g., R2 = 0.89 for Ce) and positive correlations for Mg

Landsberg laccolith formed by magma pulses 529


Table 2. Geochemistry of the Landsberg rhyolite from Halle Volcanic Complex
Sample depth [m]
29 56 76 102 128 155 175 197 201 225 245 258 281 304 328 357 378 400 428 430 452 481
SiO2 [wt%] 72.8 72.2 71.9 72.1 71.7 72.3 72.2 73.8 67.7 72.8 73.1 72.6 72.2 72.2 71.8 71.5 73.2 73.0 72.2 72.3 72.6 71.9
Al 2O 3 13.5 13.7 13.6 13.8 13.6 13.4 13.6 13.1 16.2 13.3 13.0 13.7 13.3 13.1 12.7 12.8 12.7 13.4 12.6 13.3 13.1 13.7
Fe 2O 3 2.8 2.8 3.1 2.7 2.6 2.6 2.5 2.3 3.0 2.5 2.6 2.7 2.7 2.5 2.5 2.8 2.5 2.4 2.5 2.2 2.3 2.6
MgO 0.42 0.47 0.57 0.78 0.96 1.13 0.9 0.71 0.68 0.99 0.77 0.81 0.72 0.59 0.45 0.6 0.57 0.52 0.5 1.02 0.48 0.65
CaO 0.21 0.24 0.17 0.17 0.34 0.33 0.13 0.11 0.18 0.24 0.40 0.20 0.61 0.75 1.89 1.50 0.84 0.44 1.44 0.64 0.59 0.49

530 E. S l odczyk et al.


Na 2O 2.5 2.7 2.7 2.1 2.0 2.2 1.9 3.4 3.5 3.2 3.0 3.9 2.9 2.4 4.2 3.1 3.3 3.1 3.4 2.8 3.0 2.7
K 2O 6.0 6.0 6.1 6.3 6.2 5.9 6.7 4.6 6.2 4.8 5.5 4.2 5.5 5.9 3.4 4.8 4.8 5.7 5.0 5.8 5.8 6.1
TiO2 0.23 0.23 0.24 0.22 0.21 0.22 0.21 0.19 0.25 0.21 0.20 0.21 0.22 0.21 0.20 0.19 0.20 0.20 0.22 0.21 0.20 0.23
P 2O 5 0.06 0.07 0.06 0.06 0.06 0.06 0.07 0.06 0.07 0.06 0.06 0.07 0.06 0.06 0.06 0.06 0.07 0.06 0.06 0.06 0.06 0.06
MnO <0.01 0.01 0.02 0.02 0.02 0.02 0.02 0.02 0.01 0.02 0.02 0.02 0.03 0.02 0.04 0.03 0.03 0.02 0.04 0.02 0.02 0.02
LOI 1.3 1.5 1.4 1.5 2.1 1.8 1.7 1.6 2.1 1.8 1.4 1.5 1.6 2.1 2.7 2.4 1.7 1.1 2 1.6 1.7 1.5
Total 99.8 99.9 99.8 99.8 99.8 99.9 99.9 99.9 99.9 99.9 100 99.9 99.8 99.8 99.9 99.8 99.9 99.9 99.9 99.9 99.8 99.9

Sc [ppm] 6 6 6 6 6 6 6 6 7 5 5 6 6 6 6 5 6 5 5 6 5 6
Ba 617 589 704 632 544 580 595 499 532 267 470 240 400 422 128 298 325 364 374 555 452 483
Be 2 2 3 2 4 1 <1 <1 3 <1 1 3 <1 3 <1 4 <1 <1 1 1 2 <1
Co 2.6 1.6 2.6 4 2.1 2.6 2.1 2.4 1.9 2.8 2.4 2.7 2.2 2.5 1.7 2 1.5 1.4 1.3 1.7 1.1 1.7
Cs 4.8 2.2 1.6 3 2.6 2.4 5.5 2.4 4.7 2 2 3.2 2.4 3.1 2.1 2.6 2.5 2.2 2 11.2 2.9 4.1
Ga 16.3 17.1 19.4 18.6 17.7 17.9 17.4 18.6 21.5 17.8 17.6 20.5 18.2 18.4 16.3 16.2 16.7 15.7 14.5 19.3 16.6 18.9
Hf 5.1 5.9 6.1 5.8 5.8 5.7 5.4 5.5 7 5.1 5.4 5.1 5.6 5.5 4.8 5.2 5.1 5.6 5.5 5.7 5.4 5.9
Nb 18.6 24.5 21.4 20.2 17.9 18.8 17.2 17.4 22.6 17 20.9 18.2 18.2 18.4 17.1 18.6 20.5 19.1 19.5 19.5 17.3 19.5
Rb 206 221 228 243 221 205 228 174 220 175 184 161 194 229 121 166 169 207 190 259 225 245
Sn 5 5 5 4 5 6 5 6 7 6 6 6 5 5 5 5 6 5 4 8 6 4
Sr 32.3 36 39.5 35.5 27.5 28.4 27.2 27.6 33 22.1 32.7 21.1 21.2 23.1 19.1 25 25.5 21.6 24 40.5 26.7 31
Ta 1.6 1.4 1.6 1.6 1.5 1.5 1.4 1.4 1.6 1.4 1.5 1.4 1.4 1.7 1.4 1.4 1.4 1.6 1.6 1.5 1.7 1.5
Th 18.6 18.8 19.9 17.9 18.6 17.8 18.2 18 20.8 18.4 18 16.3 18.2 18.2 16.6 16.5 16.9 18.3 17.8 17.7 18.7 19.3
U 3.7 4 3.4 5.5 3.9 4.2 4 4.2 4.9 5.6 4 5.1 7.3 4.4 14.1 3.8 3.9 5 6.6 4.7 4.7 4.5
V 29 16 29 15 16 28 20 36 17 24 10 16 96 24 15 13 19 16 15 15 27 25
W 4.1 3.9 1.7 1.8 5.5 2.3 2.3 1.8 3.3 2 2.3 2.5 2.2 1.5 2.1 2.2 2.3 2.4 3.3 3.3 3.5 8
Zr 188 216 219 204 196 194 188 200 239 172 198 188 181 187 169 185 188 193 202 184 191 208
Y 34.9 31.1 34.2 35.8 26.4 33.8 30.2 32.3 38.2 31.7 34.5 29.2 37.2 39.2 32.8 38.5 35.6 33.8 38.4 33 38.3 32.1
La 62.3 58.9 60.4 55.8 59.2 55.1 51.3 53.3 62.7 56 53.6 45.1 56.4 52.1 55.4 80.4 63.5 66.3 50.2 50.1 53.8 63.1
Ce 121 118 115 104 117 106 107 111 124 107 107 102 113 107 99 114 113 118 116 106 113 112
Pr 13.6 13 13 12.1 13.2 12 12.4 12.2 13.8 12.1 12.1 11.3 12.7 12.6 11 12.7 13 13.1 12.7 12.2 11.9 12.1
Nd 49 45.5 46.9 42.6 47 42.4 45.2 44.5 47.8 42.6 43.7 41 45.6 44.6 39.1 40.8 46 43.8 45 42.2 42.2 40.8
Sm 8.99 8.26 8.36 7.7 8.03 7.85 8.53 7.91 8.91 7.75 7.65 7.74 8.06 8.25 7.08 7.04 7.94 7.13 8.27 7.74 7.47 6.52
Eu 0.89 0.92 0.78 0.82 0.8 0.84 0.86 0.85 0.85 0.74 0.86 0.8 0.82 0.86 0.65 0.77 0.8 0.74 0.89 0.7 0.8 0.62
Gd 7.35 6.7 7.14 7 6.2 6.16 6.54 6.67 7.67 6.32 6.62 6.21 6.88 7.5 6.1 6.48 6.59 6.18 7.39 6.56 6.54 6.17
Tb 1.11 1.01 1.09 1.15 0.89 1.05 0.99 1.01 1.16 1 1.07 0.92 1.12 1.18 1.01 1.15 1.06 1.05 1.18 1.02 1.11 1
Dy 5.95 5.95 6.19 6.67 4.89 6.29 5.14 5.77 6.81 5.98 6.35 5.1 6.62 7.03 6.13 6.98 6.27 6.22 7.1 5.8 6.62 5.87
Ho 1.27 1.16 1.23 1.25 0.91 1.2 1.01 1.15 1.27 1.11 1.19 1 1.27 1.34 1.14 1.3 1.13 1.15 1.35 1.11 1.28 1.17
Er 3.21 3.29 3.55 3.66 2.51 3.44 2.97 3.51 3.74 3.37 3.38 2.83 3.58 3.99 3.35 3.78 3.3 3.38 3.84 3.19 3.63 3.5
Tm 0.54 0.48 0.53 0.54 0.4 0.49 0.43 0.5 0.57 0.47 0.52 0.44 0.54 0.61 0.49 0.56 0.49 0.52 0.54 0.5 0.55 0.48
Yb 2.99 3.16 3.23 3.46 2.63 3.15 2.69 3.22 3.64 3.15 3.38 2.77 3.44 3.66 3.2 3.57 3.21 3.21 3.32 2.96 3.48 3.35
Lu 0.46 0.46 0.49 0.53 0.4 0.48 0.41 0.44 0.53 0.43 0.49 0.42 0.52 0.54 0.48 0.55 0.47 0.48 0.5 0.46 0.5 0.49
Mo 0.4 0.5 0.5 0.3 0.3 0.3 0.4 0.3 0.3 0.4 0.4 0.4 0.3 0.5 0.3 0.5 0.3 0.7 0.5 0.6 0.7 0.5
Cu 2.1 4.6 3.1 2.5 6.3 2.4 3.7 2.8 2.1 2.1 3.7 2.1 1.6 3 1.9 5.4 5.2 2.2 2.4 5.1 3.1 2.1
Pb 3.6 2.7 2.8 3 2.7 2.9 2.5 2 3.2 3 2.6 1.6 1.7 2.4 2.7 1.7 2 2.4 4.7 6 2.9 3
Zn 15 22 30 27 26 25 25 28 19 35 26 24 25 39 6 10 16 13 19 13 17 24
Ni 2.4 2.4 4 3.5 2.3 2.5 2.4 2.7 1.5 3.2 2.6 2.5 2.2 2.8 1.8 3.8 2.2 2.3 2.8 2.4 1.9 1.8
As 2.1 1.8 1.7 1.1 1.5 1.2 1.1 5.6 1.4 1.5 1.8 1.1 0.9 1.1 1.3 2.1 0.9 0.9 1.9 1.1 0.7 0.8
Fig. 5. Correlations between major and trace elements and depth: Section 1 (left column); Sections 2 and 4 (right columm).

(R 2 = 0.91) and HREE (e.g., R2 = 0.97 for Yb). Strong Cathodoluminescence images
correlations with depth are observed in Section 3, nega- CL images of quartz show differences in the type of
tive one for Mg (R2 = 0.75) and positive one for Ca (R2 = zonation between the top (16 m) and the bottom (478 m)
0.91). This section is the only one, which shows correla- samples suggesting different sources of quartz
tions between Pl/Kfs ratio and the major and important phenocrysts in both samples. In detail the sample from
trace constituents of these two phases, i.e., Ba and Rb the top includes two types of quartz grains with different
(Fig. 6). However, the correlations are opposite to what CL zonation. Type 1 is characterized by fine oscillatory
is expected e.g., Na concentration is higher in the sam- zoning observed in whole grains (Fig. 7). The Type 1
ples with more Kfs and K, Ba and Rb in the samples con- grains are rounded and small embayments often occur at
taining more Pl (Fig. 6). the rims. The grains are also often cracked and the crack-

Landsberg laccolith formed by magma pulses 531


Fig. 6. Variations in trace elements with Pl/Kfs ratio.

ing affects whole grains suggesting that it probably oc- grow before the final emplacement of the magma as a
curred late during the crystallization history. Type 2 quartz laccolith, their varying proportions through the laccolith
zonation pattern is characterized by unzoned core sur- should represent magma portions derived from different
rounded by the zoned rim composed of only a few zones parts of a crystallizing magma plumbing system (e.g.,
(Fig. 7). The grains of Type 2 are often cracked, but not Mock et al., 2003). This fact is a strength of analyzing
rounded or embayed. Cracks in Type 2 grains occur only laccoliths for the evidence of their formation by magma
within inner core and not in the whole grains. This sug- pulses, since in plutonic magma chambers, crystals may
gests that they were formed earlier than the cracks in Type also grow in-situ and it is often difficult to recognize sev-
1 grains. eral crystal populations. Different proportions between
Sample from the bottom of laccolith include only the major phases in high silica systems may be mainly
quartz grains with one type of the CL zonation pattern. due to differences in pressure and water content and
All grains are characterized by oscillatory zoning ob- magma composition (e.g., Whitney 1975; Scaillet et al.,
served through whole grains and late cracking (Fig. 7). 1995). As such, the sections of the Landsberg laccolith
This characteristics is similar to that of the Type 1 quartz with different phenocrysts proportions could be inter-
CL pattern distinguished in the top sample. preted as different magma pulses derived from magma
sources with different composition or crystallizing in dif-
ferent conditions.
DISCUSSION
On the other hand, chemical composition of the whole
Variations with depth in the Landsberg laccolith: evidence rock is sensitive to both magmatic and alteration proc-
for many magma pulses? esses. Also, the magma differentiation may occur before
Landsberg laccolith is characterized by variations in and/or after the final emplacement. Three paths to pro-
modal and chemical composition with depth, which may duce chemical variability in a laccolith body during the
be due to the formation of the laccolith by several magma magmatic stage are by (1) in-situ mineral segregation e.g.,
pulses. The variations in proportions of phenocrysts de- by flow, (2) in-situ magma differentiation after emplace-
fine four sections in the Landsberg laccolith with differ- ment, due to preferential crystallization of background
ent Pl/Kfs ratio, however, the most consistent is the change phases in response to undercooling at the margins or (3)
in this ratio at 100 meters depth. Because phenocrysts by a coalescence of chemically different magma pulses

532 E. S l odczyk et al.


Fig. 7. Microscope and cathodoluminescence images of quartz grains from different depths (16 and 490 m) of the Landsberg
laccolith.

derived from chemically variable magma plumbing sys- vision). In detail, higher Fe, Ti, Zr and Nb contents for
tem. Since there is no evidence for flow foliation in the the top 100 m of the laccolith, which is also character-
Landsberg laccolith (Mock et al., 2005), only the latter ized by high Pl/Kfs, may suggest that this pulse was de-
two processes might have played role in the evolution of rived from a less evolved part of the crystal mush (i.e.,
magmas forming the laccolith. The chemical composi- enriched in the elements compatible in later crystallizing
tion of the analysed section of the Landsberg laccolith is accessory phases) and also could entrain more original
roughly uniform and the largest variations are observed crystals from the mush (e.g., antecrystic zircon or early
for the elements such as Ca, Mg, K, Ba, Rb, Sr and Pb, crystallized quartz as suggested by the presence of two
which are easily affected by the alteration of major phases. types of quartz grains in this section, Fig. 7). Interest-
Only the samples from the top 100 m of the laccolith show ingly, the top 100 m of the laccolith is also characterized
slightly higher contents of immobile elements such as Fe, by the highest Sr, Ba, Pb and Rb contents. These elements
Ti, Zr and Nb. This enrichment, together with a distinct may be redistributed by secondary processes, but if the
Pl/Kfs ratio in the top 100 m section of the laccolith indi- difference is magmatic in origin, such magma could be
cate that this section represents a separate magma pulse derived from a source similar to that from which fine-
and that the Landsberg laccolith was formed by at least grained rhyolites were derived, as the latter are generally
two pulses. Also, the distinct chemical composition of characterized by higher contents of these elements (Sup-
this section compared to the rest of the analysed plementary Fig. S1).
Landsberg laccolith may suggest that the magma pulses The remaining part of the analysed Landsberg laccolith
were derived from two sources. In reality, the sources (from 100 m to 480 m depth) shows no evidence for
could be separate or could occur together as ephemeral chemically different pulses as it is characterized by vari-
magma lenses in a crystallizing crystal mush (Fig. 8). Such ations only in mobile elements. However, the top 100 m
heterogeneous crustal source is consistent with the zir- of the laccolith is characterized by increases and decreases
con data from several Halle units (S l odczyk et al., in re- of certain elements with depth, including decreases in Si

Landsberg laccolith formed by magma pulses 533


Fig. 8. Schematic model of the Landsberg laccolith formation. The distribution of sedimentary rafts after: Schmiedel et al., 2015.
The emplacement of the laccolith by three magma pulses with different types of interactions between the pulses. Inset shows
secular evolution of SiO 2 in the whole rock and Pl/Kfs ratio in the phenocrysts population through the analysed section as
successive pulses form the Landsberg laccolith.

534 E. S l odczyk et al.


and LREE and increases in Al and HREE (Fig. 5). Be- depth. These correlations follow Sections borders as de-
cause we see no correlations between these elements and fined by differences in Pl/Kfs ratios suggesting in-situ
modal composition (e.g., Pl/Kfs ratio) we tentatively in- crystallization of up to 3 separate pulses in 100 to 480
terpret these variations as records of in-situ crystalliza- meter region of the Landsberg laccolith. The pulse oc-
tion of the background, probably with the lower Si melts curring between 200 and 350 meters may represent mix-
crystallizing first at the margins. Such a process could ture of magma coming from two sources: that forming
be, in theory, similar to the crystallization of chilled mar- the uppermost pulse and that forming the underlying
gins in granitic plutons, where the margins are impover- pulse.
ished in Si and the most incompatible elements. Interest-
ingly, similar correlations between Si and depth are ob- How the Landsberg laccolith was formed
served in the remaining 3 sections of the Landsberg Magma bodies grow by coalescence of many pulses
laccolith (Figs. 3 and 5) suggesting that they also repre- (Glazner et al., 2004). Separate pulses were distinguished
sent individual magma pulses recording magma differ- in magma bodies of variable size from <0.03 km3 in the
entiation as background crystallized. We believe that Si Maiden Creek sill, which was formed by 2 pulses, through
is a good marker of such a late crystallization, because the 0.05 km3 Trachyte Mesa laccolith composed of over
its content is mostly controlled by the amount of quartz 10 pulses to the 0.4 km3 Black Mesa bysmalith with un-
in the background with less quartz crystallizing in more known number of pulses (Horsman et al., 2009). From 2
undercooled regions of the pulse. In detail, Sections 2 to 4 pulses are consistent with the chemical and modal
and 4 show opposite trends in Si and some other elements analyses of the Landsberg laccolith presented in this study.
with depth (Fig. 5), which may suggest that they repre- Structural patterns and the presence of sediments in
sent a single pulse that crystallized from the top and the between separate pulses suggested that the magma bod-
bottom at the same time (Fig. 8a, inset). Also Section 3 is ies could have been formed by under-accretion, mid-ac-
characterized by low Si region at the upper contact with cretion and over-accretion of the new pulses (Menand,
Section 2 and a consistent increase in Si from the contact 2008). Formation of the laccolith by several magma pulses
with Section 4, which may indicate that Section 3 is also was also suggested for the Landsberg laccolith based on
a separate pulse that was emplaced in the middle of the the 3D and 2D geometry modeling (Schmiedel et al.,
pulse, now represented by Sections 2 and 4 (Fig. 8b, in- 2015). Our data show that modal and chemical composi-
set). The consistent change in the whole rock composi- tion of the laccoliths may offer an additional insight into
tion in Section 3 is in contrast with the variable Pl/Kfs the growth of magma bodies. In particular, modal pro-
ratio in this section, once again suggesting that the Si portions between major phenocrysts should represent
content in the whole rock is mostly controlled by the back- variations in the magma plumbing system. As the first
ground crystallization. The complex nature of Section 3 approximation the modal characteristic changes every
may be explained if the magma forming the pulse is the 100–150 meters indicating that such was the height of
mixture of the magmas forming the uppermost pulse (Sec- the magma injections, which is similar to that suggested
tion 1) with the magma forming the underlying pulse (Sec- for the Landsberg laccolith by 2D and 3D modeling
tions 2 and 4). This scenario is consistent with the posi- (Schmiedel et al., 2015). Variety in thickness of separate
tive correlation between Pl/Kfs ratio and the elements, magma pulses was observed also in other magma bodies
which are higher in Section 1, such as K, Ba, Rb and Zr. worldwide e.g., in the Maiden Creek sill (Horsman et al.,
Some of these elements are mobile, but the fact that they 2009).
correlate with Pl/Kfs ratio, which is not affected by sec- However, Section 3 in the Landsberg laccolith is com-
ondary processes, adds credence to their importance. We plex with strong variations in both modal and chemical
speculate that the correlations, if not the product of al- composition. We suggest that this is due to the injection
teration, may represent mixing between two magmas: one of new magma with a distinct chemical characteristic into
with higher Pl/Kfs, but originally also enriched in Ba, not fully solidified magma body, now represented by Sec-
Rb, Zr and K and the other with lower Pl/Kfs and con- tions 2 and 4. This process lead to magma mingling and
taining lower amounts of these elements. The mixing of interactions between the pulses (Figs. 8a and b). On the
the magmas could have happened in the plumbing sys- other hand the stronger modal and chemical contrasts
tem, on the way upwards or within the laccolith itself. between Sections 2 and 1 indicate that the latter repre-
To summarize, the combined chemical and modal data sents a magma pulse, which was over-accreted probably
from the Landsberg laccolith are consistent with the up- after the previous pulses were solid enough to avoid ex-
per 100 m of the laccolith being a separate magma pulse, tensive interactions between the pulses (Fig. 8c).
derived from a different source than the lower part of the In summary, we suggest that three successive pulses
analysed section. The evidence for more pulses comes formed the upper 500 meters of the Landsberg laccolith
from correlations between Si and other elements with (1) the first pulse that encompasses Sections 2 and 4 with

Landsberg laccolith formed by magma pulses 535


a probable overall thickness of 300 m, (2) the second pulse four sections with different Pl/Kfs ratio. For quickly
that encompasses Section 3 and was injected in the mid- cooled laccolith bodies, the variations in phencrysts pro-
dle of the pulse 1 with the thickness of approximately portions should represent different magma pulses, as such
150 m and (3) the third pulse that encompasses Section 1 variations could not develop in-situ. This division in 4
(100 m in thickness) and was over-accreted on the previ- sections was not supported by the general variations in
ous pulses (Fig. 8). We believe that the Landsberg the whole rock composition, partly because the composi-
laccolith with its relatively small volume and the high tion was affected by secondary processes and partly be-
emplacement level, which imply quick cooling, preserved cause the rhyolitic magma was chemically uniform. In
records of successive magma pulses and interaction be- fact, the variations in immobile elements were slight and
tween them from extensive interaction to limited one. mostly observed between the uppermost section and the
Our model is consistent with previous 2D and 3D remaining part of the laccolith. However, the detailed
emplacement models of the Halle laccoliths (Schmiedel analyses of variations in Si and other elements within the
et al., 2015), which also suggests pulsed model for the sections are consistent with the formation of the
formation of the Landsberg laccolith. However, Schmiedel Landsberg laccolith by three magma pulses, derived prob-
et al. (2015) also describe two major shear zones in the ably from at least two magma sources. The pulses were
laccolith at approximately 150 and 270 meters depth, the emplaced both before and after the previous pulses were
depths which are not consistent with the division based solidified leading to formation of complex variations in
on chemical and modal compostion. It is possible that mineral and chemical composition with depth. Our re-
some shear zones are not present in the core record, as in sults are consistent with 3D and 2D modeling of the ge-
many parts of the core several meter long sections were ometry of the Landsberg laccolith (Schmiedel et al.,
not recovered. However, the shear zones at 150 and 270 2015), but also offer the additional information on sources
meters should represent margins of the separate pulses of the magma pulses.
and they are just in the middle of our suggested pulses.
The complex nature of the third pulse in our model (Fig. Acknowledgments—This work was funded by National Sci-
8b, Section 3 in Fig. 3a) may suggest that it is actually ence Centre grant PRELUDIUM (UMO-2013/09/N/ST10/
composed of two or more smaller pulses and the shear 00655) to ES. AP acknowledges MOBILITY grant. Many thanks
zone at 270 meters is a part of this complexity. The dis- go to the WISMUT GmbH for allowing access and sampling of
drill cores and to Jens Götze for CL images. We thank Sven
crepancy between our contacts of pulses at 100 and 200
Morgan and anonymous reviewer for constructive reviews.
meters and the presence of the shearing zone at 150 m is
more difficult to explain and will remain the unsolved
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Figure S1
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Landsberg laccolith formed by magma pulses 537

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