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Tham Nguyen-Chung,1 Gabor Juttner,2 Cindy Loser,1 Tung Pham,3 Michael Gehde1
1
Chemnitz University of Technology, D-09107 Chemnitz, Germany
2
INTRODUCTION
Microinjection molding is nowadays seen as the most
efcient technology for large-scale manufacturing of therPresented in part at the XVth International Congress on Rheology, 2008,
Monterey, California.
Dedicated to Prof. Dr.-Ing. G. Mennig on the occasion of his 70th birthday.
Correspondence to: Tham Nguyen-Chung; e-mail: tham.nguyen.chung@
mb.tu-chemnitz.de
DOI 10.1002/pen.21536
Published online in Wiley InterScience (www.interscience.wiley.com).
C 2009 Society of Plastics Engineers
V
EXPERIMENTS
Material Data
Two grades of isotactic polypropylene (HC600TF and
DM55 pharm) with different viscosities and crystallinity
166 POLYMER ENGINEERING AND SCIENCE-2010
Z0
1
Z0 1n
t g
(1)
A1 T T
;
Z0 D1 exp
A2 T T
(2)
T D2 D3 p;
(3)
A2 A~2 D3 p;
(4)
where n, t*, D1, D2, D3, A1, and A~2 are data-tted coefcients: n 0.2336, s* 36932.7 Pa, D1 1.1233 3 1017
Pa s, D2 263.15 K, D3 1.5 3 1027 K/Pa, A1
37.761, and A~2 5 51:6 K.
The pvT data were approximated by using the Tait
model [21]:
p
ut T; p; (5)
uT; p u0 T 1 C ln 1
BT
where u(T, p) is the specic volume at temperature T and
pressure p, u0(T) is the specic volume at zero gauge
pressure, C is a constant (C 0.0894), and B accounts
for the pressure sensitivity of the material and as dened
below.
The upper temperature region (T Tt) can be described
by the equations:
u0 T b1m b2m T b5 ;
(6)
BT b3m expb4m T b5 ;
(7)
ut T; p 0;
(8)
279.2
258.9
238.7
197.6
177.6
157.7
138.5
118.3
98.3
78.2
58.5
38.8
0.1697
0.1676
0.1639
0.1547
0.1556
0.1552
0.2244
0.2267
0.2329
0.2371
0.2368
0.2442
FIG. 1. Micro-spiral.
(9)
BT b3s expb4s T b5 ;
(10)
ut T; p b7 expb8 T b5 b9 p;
(11)
where b1s, b2s, b3s, b4s, b5, b7, b8, and b9 are data-tted
coefcients.
The transition temperature Tt is a linear function of the
pressure:
Tt p b5 b6 p:
(12)
Part Geometries
Two different geometries were used: the micro-spiral
(Fig. 1) and the micro-plate (Fig. 2). The micro-spiral has
a ow length of 32 mm and a width of 1.5 mm. Two different thicknesses (0.2 mm and 0.5 mm) are available.
The micro-plate is a rectangular geometry of 12 mm 3
11 mm 3 0.5 mm. For both dimensions, the cavity is fed
from a conical sprue. The sprue and the part cavity are
connected through a junction zone.
Molding
Molding operations were conducted with a plunger
injection molding machine (formicaPlast) developed by
the Kunststoff-Zentrum in Leipzig (Germany) [22]. The
injection unit consists of a pre-plasticizing plunger and an
injection plunger (Fig. 3). The diameter of the injection
280
192
125
118
114
111
108
105
102
98
89
60
32
3030
2851
2572
2897
4349
7709
17,814
9404
3441
2661
2390
2033
1762
DOI 10.1002/pen
FIG. 2. Micro-plate.
SIMULATION
Model Geometries
plunger is 3 mm, and a fast electrical drive is used, ensuring a high precision of control for the injection speed and
the plunger position. The maximum injection pressure and
injection rate of the machine are 300 MPa and 3.5 cm3/s,
respectively.
Short-shots of different lling degrees (Fig. 4) were
produced by adopting different stop positions for the
injection plunger. Five shots were made for each set of
the processing parameters. The melt and mold temperatures as well as the plunger speed in the short-shot experiments were varied as shown in Table 3. No packing pressure was applied. The cavity pressure was measured by
using a miniaturized quartz sensor (KISTLER 6183AE).
The pressure sensor was located at the junction zone
between the sprue and the part cavity (Fig. 5) for both
part geometries.
Figure 6 shows the cavity pressure for short-shots with
10 different stop positions of the plunger. For every
plunger stop position ve short-shots were conducted,
resulting in a total number of 50 for the pressure curves.
The corresponding pressure curves of the same plunger
stop position are almost identical except for the last segments of the curves, which indicated a high degree of
reproducibility of the experiments. Average values of the
maximum pressure and the lling degree were obtained
Three-dimensional lling simulations for the micro-spiral and the micro-plate were conducted by using the software Moldow Plastics Insight (version 6.1; revision 3
was used for the micro-spiral and version 6.2, revision 2
for the micro-plate).
Only half of the actual cavity was taken into account
(Fig. 7) in cases of the micro-spiral geometry. The symmetry surface was considered as a usual mold wall with a
no-slip condition applied being an acceptable simplication as a result of the fact that the dimensions of the
junction zone are much larger compared with the thickness of the spiral region. The conical sprue was not
included in the model because the ow resistance in the
sprue is much smaller than the one in the spiral and
therefore can be neglected. This allows the calculated
injection pressure to be related to the cavity pressure
measured at the junction zone between the sprue and the
micro-spiral (Fig. 5).
In case of the micro-plate, the whole cavity including
the sprue was considered (Fig. 8) because the pressure
loss in the sprue cannot be negligible as compared with
the pressure loss in the micro-plate. The pressure level in
the micro-plate is much lower than in the micro-spirals,
as can be seen later in the results.
Governing Equations
The governing equations used in the software are the
conservation equations of mass, momentum, and energy
[23]:
qr
r r~
u 0
(13)
qt
Dr~
u
rp r t
Dt
(14)
DOI 10.1002/pen
No.
Material
Geometry
d
(mm)
Tmold
(8C)
Tmelt
(8C)
vP
(mm/s)
1
2
3
4
5
6
7
8
9
10
11
12
13
14
15
16
HC600TF
Micro-spiral
0.2
20/30a
280
20
50
100
200
20
50
100
200
50
100
150
200
50
100
150
200
DM55 pharm
Micro-plate
0.5
20/30a
280
0.5
70
220
280
rcp
DT
Dp
bT
r krT Zg2
Dt
Dt
(15)
where t, ~
t, T, p, s; c_ , q, g, cp, b, and k denote time, velocity vector, temperature, pressure, stress tensor, shear rate,
density, viscosity, specic heat, expansivity, and thermal
conductivity, respectively.
For the constitutive equation, the generalized Newtonian uid model is assumed [23]:
t 2Zg ; T; pg
(16)
1
r~
u r~
uT
2
(17)
DOI 10.1002/pen
size on the surface for the part was set to 0.1 mm, and at
least 12 layers of tetrahedra were needed along the spiral
thickness. The mesh of the micro-spiral part consisted of
about 500,000 tetrahedral elements in total. Similarly, the
maximal increase of the volume between two successive
time steps was reduced from the default value of 4% to
0.025% of the cavity volume.
RESULTS
Figure 10 shows the relationship between the injection
pressure and the lling degree for the micro-spirals with a
thickness of 0.2 mm. The experiments were done with a
plunger speed varying between 20 mm/s and 200 mm/s,
while all other processing parameters were kept constant.
For injection speeds between 50 mm/s and 200 mm/s, the
experimental data can be properly tted by the simulation
by using values of the heat transfer coefcient between
25,000 W/m2K and 1500 W/m2K.
The heat transfer coefcient value of 25,000 W/m2K
seems, at rst glance, to be very high, but not unrealistic.
In the older versions of the Moldow software, this value
FIG. 10. Pressure vs. lling degree for the micro-spirals with a thickness of 0.2 mm.
FIG. 11. Pressure vs. lling degree for the micro-spirals of 0.2 mm
thickness for the lowest injection speed.
DOI 10.1002/pen
FIG. 13. Temperature distribution in the middle layer of the micro-spiral at three different times of the lling process.
FIG. 15. Pressure vs. lling degree for the micro-plates, Tmelt
2808C.
DOI 10.1002/pen
FIG. 14. Pressure vs. lling degree for the micro-spirals with a thickness of 0.5 mm.
FIG. 16. Pressure vs. lling degree for the micro-plates, Tmelt
2208C.
FIG. 18. Volume rate vs. lling degree for the micro-spirals with a
thickness of 0.2 mm.
with the one in the micro-spiral cavity and gives less variation of the heat transfer coefcient.
If a melt temperature of 2208C instead of 2808C was
applied for the micro-plates, the heat transfer coefcient
took values between 5000 W/m2K and 1500 W/m2K (Fig.
16). The heat transfer coefcient decreased, although the
pressure level in the cavity was slightly higher than in
case of the higher melt temperature of 2808C. This can be
explained by the higher viscosity of the melt. The higher
viscosity requires higher pressure to overcome the roughness at the mold surface (Fig. 17) to establish the same
level of thermal contact as compared with the previous
case. The roughness of the mold surface is also the
reason for the pressure dependency of the heat transfer
coefcient.
Figure 18 shows the volume rates calculated for the
micro-spirals with a thickness of 0.2 mm when different
plunger speeds were applied. As the melt lled the sprue
and the junction zone, the volume rates at the injection
location were equal to the theoretical values, resulting
from the plunger speed and the cross section of the
FIG. 17. Contact reduction due to the surface roughness of the mold.
CONCLUSIONS
It can be shown that the heat transfer coefcient
between the polymer and the mold wall has a signicant
inuence on the simulation results. By using precise material data and considering the melt compression in the
barrel, the actual volume rate and the temperature of the
melt at the entrance of the cavity can be correctly calculated. It was able to determine the heat transfer coefcient
by means of reverse engineering based on the relationship
between the cavity pressure and the lling degree. The
heat transfer coefcient increases by decreasing cavity
thickness or injection speed. It is believed that the pressure level in the cavity is mostly responsible for the thermal contact between the polymer and the mold wall. A
pressure-dependent model for the heat transfer coefcient
would be more suitable to describe the thermal contact
behavior in microinjection molding, especially in case of
micro-cavities of high aspect ratio.
To take this phenomenon into consideration in the
numerical simulation, three different aspects have to be
considered: surface roughness of the mold, material propDOI 10.1002/pen
DOI 10.1002/pen
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